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1.
Sci Total Environ ; 931: 172857, 2024 Apr 30.
Artigo em Inglês | MEDLINE | ID: mdl-38692318

RESUMO

Residential natural gas meter set assemblies (MSAs) emit methane (CH4), but reported emissions factors vary. To test existing emissions factors, we quantified CH4 emissions from 37 residential MSAs in Calgary, Alberta, Canada. A notable difference with previous studies is the targeted measurement of regulator vents in this study, which were measured with a static chamber, while fugitives were measured with a modified hi-flow sampler. Emissions were dominated by pressure regulator vents (emissions factor = 1.18 g CH4/h/MSA), but 7 fugitives were found (emissions factor = 0.018 g CH4/h/MSA). Six regulator vents were emitting at notably higher rates (≥ 1.79 g CH4/h/MSA). The total empirical emissions factor was 1.20 g CH4/h/MSA (95 % CI, 1.03 to 1.37 g/h/MSA). This is ∼7 times higher than the emissions factor for residential MSAs used in the U.S. EPA's Greenhouse Gas Inventory, which may not include emissions from regulator vents. Upscaling to annual CH4 emissions in Calgary indicates 3234.6 t CH4/yr (95 % CI, 2776.4 t to 3692.9 t CH4/yr) could be emitted from MSAs. This is equivalent to 4.1 % (95 % CI, 3.5 % to 4.7 %) of total city-level CH4 emissions as estimated with satellite data. Results suggest residential MSA emissions may be under-estimated and further study isolating root causes of regulator vent emissions is required to guide mitigation and improve emissions modeling.

2.
Sci Rep ; 13(1): 16759, 2023 Oct 05.
Artigo em Inglês | MEDLINE | ID: mdl-37798261

RESUMO

Satellite observations have been used to measure methane (CH4) emissions from the oil and gas (O&G) industry, particularly by revealing previously undocumented, very large emission events and basin-level emission estimates. However, most satellite systems use passive remote sensing to retrieve CH4 mixing ratios, which is sensitive to sunlight, earth surface properties, and atmospheric conditions. Accordingly, the reliability of satellites for routine CH4 emissions monitoring varies across the globe. To better understand the potentials and limitations of routine monitoring of CH4 emissions with satellites, we investigated the global observational coverage of the TROPOMI instrument onboard the Sentinel-5P satellite-the only satellite system currently with daily global coverage. A 0.1° × 0.1° gridded global map that indicates the average number of days with valid observations from TROPOMI for 2019-2021 was generated by following the measurement retrieval quality-assurance threshold (≥ 0.5). We found TROPOMI had promising observational coverage over dryland regions (maximum: 58.6%) but limited coverage over tropical regions and high latitudes (minimum: 0%). Cloud cover and solar zenith angle were the primary factors affecting observational coverage at high latitudes, while aerosol optical thickness was the primary factor over dryland regions. To further assess the country-level reliability of satellites for detecting and quantifying CH4 emissions from the onshore O&G sector, we extracted the average annual TROPOMI observational coverage (TOC) over onshore O&G infrastructure for 160 countries. Seven of the top-10 O&G-producing countries had an average annual TOC < 10% (< 36 days per year), which indicates the limited ability to routinely identify large emissions events, track their duration, and quantify emissions rates using inverse modelling. We further assessed the potential performance of the latter by combining TOC and the uncertainties from the global O&G inventory. Results indicate that the accuracy of emissions quantifications of onshore O&G sources using TROPOMI data and inverse modeling will be higher in countries located in dryland and mid-latitude regions and lower in tropical and high-latitude regions. Therefore, current passive-sensing satellites have low potential for frequent monitoring of large methane emissions from O&G sectors in countries located in tropical and high latitudes (e.g., Canada, Russia, Brazil, Norway, and Venezuela). Alternative methods should be considered for routine emissions monitoring in these regions.

3.
Sensors (Basel) ; 23(10)2023 May 16.
Artigo em Inglês | MEDLINE | ID: mdl-37430713

RESUMO

There are two primary algorithms for autonomous multiple odor source localization (MOSL) in an environment with turbulent fluid flow: Independent Posteriors (IP) and Dempster-Shafer (DS) theory algorithms. Both of these algorithms use a form of occupancy grid mapping to map the probability that a given location is a source. They have potential applications to assist in locating emitting sources using mobile point sensors. However, the performance and limitations of these two algorithms is currently unknown, and a better understanding of their effectiveness under various conditions is required prior to application. To address this knowledge gap, we tested the response of both algorithms to different environmental and odor search parameters. The localization performance of the algorithms was measured using the earth mover's distance. Results indicate that the IP algorithm outperformed the DS theory algorithm by minimizing source attribution in locations where there were no sources, while correctly identifying source locations. The DS theory algorithm also identified actual sources correctly but incorrectly attributed emissions to many locations where there were no sources. These results suggest that the IP algorithm offers a more appropriate approach for solving the MOSL problem in environments with turbulent fluid flow.

5.
Sci Rep ; 11(1): 12092, 2021 06 08.
Artigo em Inglês | MEDLINE | ID: mdl-34103585

RESUMO

Small aerial drones are used in a growing number of commercial applications. However, drones cannot fly in all weather, which impacts their reliability for time-sensitive operations. The magnitude and global variability of weather impact is poorly understood. We explore weather-limited drone flyability (the proportion of time drones can fly safely) by comparing historical wind speed, temperature, and precipitation data to manufacturer-reported thresholds of common commercial and weather-resistant drones with a computer simulation. We show that global flyability is highest in warm and dry continental regions and lowest over oceans and at high latitudes. Median global flyability for common drones is low: 5.7 h/day or 2.0 h/day if restricted to daylight hours. Weather-resistant drones have higher flyability (20.4 and 12.3 h/day, respectively). While these estimates do not consider all weather conditions, results suggest that improvements to weather resistance can increase flyability. An inverse analysis for major population centres shows the largest flyability gains for common drones can be achieved by increasing maximum wind speed and precipitation thresholds from 10 to 15 m/s and 0-1 mm/h, respectively.

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